I've written a very simple application to test this method (besides just testing the example given on that page) and have now embarked on something larger following the same process.
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I think this is already possible for Perl, using the Tcl::Tk CPAN module.
Vtcl is used just for GUI layout, widgets are bound by their aliases in a Perl script, then the same Perl script is used for functionality.
Here's a page talking about it:
http://vkonovalov.ru/vtcl-usage/Using_vtcl_for_creating_Tcl-Tk_GUI_for_Perl.html
I've written a very simple application to test this method (besides just testing the example given on that page) and have now embarked on something larger following the same process.